国产 CF/PEEK 预浸料激光辅助自动铺缠工艺及力学性能

曾丹 ,  李勇 ,  吴悦梅 ,  易磊隽 ,  李彩林

航空材料学报 ›› 2026, Vol. 46 ›› Issue (7) : 151 -162.

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航空材料学报 ›› 2026, Vol. 46 ›› Issue (7) : 151 -162. DOI: 10.11868/j.issn.1005-5053.2025.000125

国产 CF/PEEK 预浸料激光辅助自动铺缠工艺及力学性能

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Laser-assisted automated lay-up process and mechanical properties of domestic CF/PEEK prepregs

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摘要

CF/PEEK 复合材料是适用于极端环境的战略材料,但因 PEEK 树脂加工难度大、国产预浸料制备及自动铺放技术尚不成熟,制约着其广泛的工程化应用。本工作基于自研的预浸料拉制设备和纤维自动铺放平台,系统开展国产 CF/PEEK 预浸料自主制备与工艺研究。首先,采用粉末浸渍法制备 CF/PEEK 预浸料,再通过自动铺缠正交实验揭示成型温度、压力和绕速对制件性能的影响规律。结果表明:制备的预浸料符合自动铺放工艺要求,铺放过程各因素对制件性能的影响程度排序:温度>绕速>压力,最佳成型工艺参数组合:激光功率 220 W,气动压力 0.3 MPa,铺缠速率 101 mm/s,此时层间剪切强度 55.7 MPa,拉伸强度 2006.4 MPa,分别达到热压件的 84.7%、86.7%,孔隙率为 3.4%。通过与国外相关研究对比,分析影响性能的主要原因在于材料性能、工艺控制及装备水平等方面的差距。本工作研究可为国产化的材料-装备-工艺技术体系化开发提供参考。

Abstract

CF/PEEK composite are strategic materials suitable for extreme environments. However, the difficulty in processing PEEK resin, the immaturity of domestic prepreg preparation and automated placement technology restrict its widespread engineering application. This study systematically investigates the preparation and lay-up processes of domestically produced CF/PEEK prepreg using self-developed prepreg pulling equipment and an automated fiber placement platform. First, CF/PEEK prepregs are fabricatedvia the powder impregnation method. Subsequently, orthogonal experiments are conducted to evaluate the effects of lay-up temperature, pressure and speed on the properties of the fabricated components. The results demonstrate that the prepared prepreg meets the requirements for automated lay-up. The influence of process parameters on part performance follows the order: temperature > lay-up speed > pressure. The optimal parameter combination is identified as: laser power of 220 W, pneumatic pressure of 0.3 MPa and lay-up speed of 101 mm/s. Under these conditions, the composites achieve an interlaminar shear strength of 55.7 MPa and a tensile strength of 2006.4 MPa, reaching 84.7% and 86.7% of the performance of hot-pressed counterparts, respectively, with a porosity of 3.4%. By comparing with relevant foreign research, the underlying causes of performance gaps are analyzed. This study provides reference for the systematic development of domestically produced materials, equipment and process technologies.

关键词

CF/PEEK / 热塑性复合材料 / 自动铺放技术 / 工艺参数 / 层间剪切强度

Key words

CF/PEEK / thermoplastic composite / automated fiber placement technology / process parameter / interlaminar shear strength

引用本文

引用格式 ▾
曾丹,李勇,吴悦梅,易磊隽,李彩林. 国产 CF/PEEK 预浸料激光辅助自动铺缠工艺及力学性能[J]. 航空材料学报, 2026, 46(7): 151-162 DOI:10.11868/j.issn.1005-5053.2025.000125

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参考文献

[1]

SONMEZ F O, AKBULUT M. Process optimization of tape placement for thermoplastic composites[J].Composites Part A, 2007, 38(9): 2013-2023.

[2]

PITCHUMANI R, GILLESPIE J W, LAMONTIA M A. Design and optimization of a thermoplastic tow—placement process with in—situ consolidation[J].Journal of Composite Materials, 1997, 31(3): 244-275.

[3]

霍红宇, 姚鑫, 高亮, . 高性能连续纤维增强热塑性预浸料及复合材料制备工艺研究进展[J].材料工程, 2025, 53(3): 44-53.

[4]

HUO H Y, YAO X, GAO L, et al. Research progress in preparation technology of high performance continuous fiber reinforced thermoplastic prepreg and its composites[J].Journal of Materials Engineering, 2025, 53(3): 44-53.

[5]

任毅, 虞筱琛, 祝颖丹, . 碳纤维增强热塑性复合材料激光原位成型工艺调控研究进展[J].塑料工业, 2025, 53(2): 6-12.

[6]

REN Y, YU X C, ZHU Y D, et al. Research progress on regulations of laser in—situ consolidation processes for carbon fiber reinforced thermoplastic composites[J].China Plastics Industry, 2025, 53(2): 6-12.

[7]

AGUST Z, OSTRANDER G, MICHASIOW J, et al. Recent developments in automated fiber placement of thermo—plastic composites[J].SAMPLE Journal, 2014, 50(2): 30-35.

[8]

AGARWAL V, GUCERI S I, MCCULLOUGH R L, et al. Thermal characterization of the laser—assisted consolidation process[J].Journal of Thermoplastic Composite Materials, 1992, 5(2): 115-135.

[9]

ROSSELLI F, SANTARE M H, GÜÇERI S I. Effects of processing on laser assisted thermoplastic tape consolidation[J].Composites Part A, 1997, 28(12): 1023-1033.

[10]

SCHLOTTERMÖLLER M, SCHLEDJEWSKI R, MITSCHANG P. Influence of process parameters on residual stress in thermoplastic filament—wound parts[J].Journal of Material, 2004, 218(2): 157-164.

[11]

QUADRINI F, SQUEO E A, PROSPERI C. Diode laser assisted filament winding of thermoplastic matrix composites[J].Materials, 2010, 3(1): 563-571.

[12]

COMER A J, RAY D, OBANDE W O, et al. Mechanical characterisation of carbon fibre—PEEK manufactured by laser—assisted automated—tape—placement and autoclave[J].Composites Part A, 2015, 69: 10-20.

[13]

STOKES—GRIFFIN C M, COMPSTON P. The effect of processing temperature and placement rate on the short beam strength of carbon fibre—PEEK manufactured using a laser tape placement process[J].Composites Part A, 2015, 78: 274-283.

[14]

ÇELIK O, CHOUDHARY A, PEETERS D, et al. Deconsolidation of thermoplastic prepreg tapes during rapid laser heating[J].Composites Part A, 2021, 149: 106575.

[15]

OROMIEHIE E, GAIN A K, PRUSTY B G. Processing parameter optimisation for automated fibre placement (AFP) manufactured thermoplastic composites[J].Composite Structures, 2021, 272: 114223.

[16]

SHAFAQ, DONOUGH M J, FARNSWORTH A L, et al. Influence of deposition rates on the mode Ⅰ fracture toughness of in—situ consolidated thermoplastic composites[J].Composites Part B, 2023, 251: 110474.

[17]

POURAHMADI E, SHADMEHRI F, GANESAN R. Interlaminar shear strength of carbon/PEEK thermoplastic composite laminate: effects of in—situ consolidation by automated fiber placement and autoclave re—consolidation[J].Composites Part B, 2024, 269: 111104.

[18]

SHAFAQ S, DONOUGH M J, BHANDARI B, et al. Experimental study on the influence of optimised automated fibre placement processing parameters on the impact response and residual flexural strength of AS4/APC—2 laminates[J].Composites Science and Technology, 2025, 259: 110945.

[19]

唐邦铭. 热塑性预浸带缠绕工艺参数及加热方式对成型质量及内应力的影响[J].复合材料学报, 1999, 16(2): 21-28.

[20]

TANG B M. Influence of winding parameters and of heating systems with thermoplastic tape on qualities and internal stresses of a part[J].Acta Materiae Compositae Sinica, 1999, 16(2): 21-28.

[21]

张昕, 李辅安, 王晓洁. 热塑性树脂基体纤维缠绕工艺[J].纤维复合材料, 2003, 20(1): 27-29.

[22]

ZHANG X, LI F A, WANG X J. Thermoplastic filament winding[J].Fiber Composites, 2003, 20(1): 27-29.

[23]

方立, 周晓东. 连续纤维增强热塑性复合材料的浸渍及其缠绕成型[J].纤维复合材料, 2008, 25(3): 27-31.

[24]

FANG L, ZHOU X D. Impregnation and filament winding of continuous fiber reinforced thermoplastic composites[J].Fiber Composites, 2008, 25(3): 27-31.

[25]

韩振宇, 孙守政, 付云忠, . 热塑性 FRP 自动铺放成型缺陷的多尺度研究进展[J].材料工程, 2017, 45(7): 118-127.

[26]

HAN Z Y, SUN S Z, FU Y Z, et al. Multi—scale research progress of manufacturing defects for thermoplastic FRP fabricated by automated fiber placement[J].Journal of Materials Engineering, 2017, 45(7): 118-127.

[27]

李靖, 洪成, 郭兵兵, . 铺放成型工艺参数对复合材料板材弯曲强度和层间剪切强度的影响[J].玻璃钢/复合材料, 2017(5): 72-79.

[28]

LI J, HONG C, GUO B B, et al. Study on processing parameters of tape placement for continuous GF reinforced PPS[J].Fiber Reinforced Plastics/Composites, 2017(5): 72-79.

[29]

宋清华, 刘卫平, 肖军, . 热塑性复合材料自动铺放工艺参数分析与优化[J].复合材料学报, 2018, 35(5): 1149-1157.

[30]

SONG Q H, LIU W P, XIAO J, et al. Analysis and optimization of the processing parameters for automated fiber placement of thermoplastic composites[J].Acta Materiae Compositae Sinica, 2018, 35(5): 1149-1157.

[31]

吴瑶平. 热塑性复合材料缠绕过程温度场分析及工艺参数优化研究[D].南京: 南京航空航天大学, 2018.

[32]

WU Y P. Research on temperature field and parameter optimization for thermoplastic composite winding process[D]. Nanjing:Nanjing University of Aeronautics and Astronautics, 2018.

[33]

梁宜楠. CF/PEEK 点阵结构自动铺放原位成型工艺研究[D].大连: 大连理工大学, 2021.

[34]

LIANG Y N. Automated fiber placement and in—situ consolidation process of CF/PEEK lattice structure[D]. Dalian:Dalian University of Technology, 2021.

[35]

DONG N G, LUAN C C, YAO X H, et al. Influence of process parameters on the interlaminar shear strength of CF/PEEK composites in—situ consolidated by laser—assisted automated fiber placement[J].Composites Science and Technology, 2024, 258: 110902.

[36]

JIANG W, CHEN C, CHEN Z K, et al. Effect of crystallinity on optical properties of PEEK prepreg tapes for laser—assisted automated fiber placement[J].Composites Communications, 2023, 38: 101490.

[37]

ZHANG C P, DUAN Y G, XIAO H, et al. Effect of porosity and crystallinity on mechanical properties of laser in—situ consolidation thermoplastic composites[J].Polymer, 2022, 242: 124573.

[38]

蒋威. 热塑性复合材料自动铺放过程激光加热机理与温度场优化[D].武汉: 华中科技大学, 2024.

[39]

JIANG W. Laser heating mechanism and temperature field optimisation for automated fiber placement process of thermoplastic composites[D]. Wuhan:Huazhong University of Science and Technology, 2024.

[40]

董晨华. 热塑性复合材料原位固结变形机理及工艺调控[D].大连: 大连理工大学, 2021.

[41]

DONG C H. Deformation mechanism and process control of in—situ consolidation of thermoplastic composites[D]. Dalian:Dalian University of Technology, 2021.

基金资助

成都航空职业技术大学校级自然科研基金项目(ZZX0624110)

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